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          Prompt Fission Neutron Spectra of Actinides

          Closed for Proposals

          Project Type

          Coordinated Research Project

          Project Code

          F41026

          CRP

          1673

          Approved Date

          6 November 2009

          Project Status

          Closed

          Start Date

          6 November 2009

          Expected End Date

          30 April 2015

          Completed Date

          29 October 2014

          Description

          The energy spectrum of prompt neutrons emitted in fission plays an important role in many applications in nuclear science and technology. The Co-ordinated Research Project on “Prompt fission neutron spectra of actinides” is proposed to provide prompt fission neutron spectra for 235,238U, 239Pu and 232Th nuclei. The outcome would be a recommended evaluation of prompt fission spectra of major actinides with covariances from thermal to 20 MeV incident neutrons, including validation against integral critical assembly and dosimetry data. Reactor operators and designers will draw upon data generated from this CRP to improve both operational safety and efficiency. Modelling efforts will use these data in diagnosing reactors and critical devices and in optimising design parameters in future reactor.s

          Objectives

          To enhance the ability of MS to produce and/or utilise good quality nuclear data in their existing reactor applications’ databases through evaluation of prompt fission neutron spectra with covariances from thermal to 20 MeV for major actinides

          Specific Objectives

          To facilitate interaction and sharing of work within the community in a timely and professional manner

          To incorporate available experimental information on PFNS for major actinides into evaluated nuclear data files

          To make available existing experimental information on prompt fission neutron spectra (PFNS) relevant to fission reactors’ applications, which can be processed and used by users worldwide,

          To recommend evaluations of PFNS with covariances from thermal to 20 MeV incident neutron energy

          Impact

          This CRP produced key evaluations of the prompt fission neutron spectra for major actinides which have been adopted in national and international evaluated nuclear libraries worldwide.
          The CRP has been extremely successful. A highly cited comprehensive technical paper was published summarizing the CRP results.

          Relevance

          Highly relevant to improve the evaluated PFNS data.

          CRP Publications

          USA, France, Slovenia, Russia, The Netherlands, Austria, UK, IAEA: M.B. Chadwick et al
          Peer-reviewed paper international journal
          Nuclear Data Sheets, Volume 112, Issue 12, December 2011, Pages 2887-2996
          ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data
          IRMM: A. Al-Adili, F.-J. Hambsch, S. Pomp, S. Oberstedt
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 158-164
          Indication of anisotropic TKE and mass emission in 234U(n,f)
          IRMM and Ohio University, USA:
          Peer-reviewed paper international journal
          NUCLEAR SCIENCE AND ENGINEERING: 168, 73–74 (2011)
          Absolute Ratio 252Cf to 235U Prompt Fission Neutron Spectra
          IRMM, KFKI, Hungary, IAEA/NDS: N. KORNILOV, F.-J. HAMBSCH, I. FABRY, S. OBERSTEDT, T.BELGYA, Z. KIS, L. SZENTMIKLOSI, and S. SIMAKOV,
          Peer-reviewed paper international journal
          NUCLEAR SCIENCE AND ENGINEERING 165, 117 (2010)
          The 235U(n,f) Prompt Fission Neutron Spectrum at 100 K Input Neutron Energy
          USA, France, Slovenia, Russia, The Netherlands, Austria, UK, IAEA: M.B. Chadwick et al
          Peer-reviewed paper international journal
          Nuclear Data Sheets, Volume 112, Issue 12, December 2011, Pages 2887-2996
          ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data
          LANL (USA): Patrick Talou, Mike Rising, Toshihiko Kawano and Anil Prinja
          Peer-reviewed paper international journal
          EPJ Web of Conferences 27, 00001 (2012)
          Systematic Quantification of Uncertainties for Evaluated Prompt Fission Neutron Spectra and Multiplicities
          LANL (USA): E. Kwan, C.Y. Wu, R.C. Haight, H.Y. Lee, T.A. Bredeweg, A. Chyzh, M. Devlin, N. Fotiades, J.M. Gostic, R.A. Henderson, M. Jandel, A. Laptev, R.O. Nelson, J.M. O'Donnell, B.A. Perdue, T.N. Taddeucci, J.L. Ullmann, S.A. Wender
          Peer-reviewed paper international journal
          Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Volume 688, 1 October 2012, Pages 55-61
          Prompt energy distribution of 235U(n,f) at bombarding energies of 1–20 MeV
          CEA (France) : Olivier Litaize, Olivier Serot, David Regnier, Stephane Theveny, Sebastien Onde,
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 51-58
          New Features of the FIFRELIN Code for the Investigation of Fission Fragments Characteristics
          IRMM; A. Al-Adili, F.-J. Hambsch, S. Pomp, and S. Oberstedt
          Peer-reviewed paper international journal
          Phys. Rev. C 86, 054601 – Published 5 November 2012
          Impact of prompt-neutron corrections on final fission-fragment distributions
          Romania, IRMM: A. Tudora, C. Morariu, F.-J. Hambsch, S. Oberstedt, C. Manailescu,
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 43-50
          Prompt Gamma-ray Energy in the Frame of Prompt Neutron Emission Models
          Romania, IRMM: C. Manailescu, A. Tudora, F.-J. Hambsch, C. Morariu, S. Oberstedt
          Peer-reviewed paper international journal
          Nuclear Physics A, Volume 867, Issue 1, 1 October 2011, Pages 12-40
          Possible reference method of total excitation energy partition between complementary fission fragments
          Romania, IRMM: A. Tudora, F.-J. Hambsch, S. Oberstedt
          Peer-reviewed paper international journal
          Nuclear Physics A, Volumes 890–891, 1 October 2012, Pages 77-101
          Sub-barrier resonance fission and its effects on fission fragment properties
          IRMM, KFKI, Hungary, IAEA/NDS: N. KORNILOV, F.-J. HAMBSCH, I. FABRY, S. OBERSTEDT, T.BELGYA, Z. KIS, L. SZENTMIKLOSI, and S. SIMAKOV,
          Peer-reviewed paper international journal
          NUCLEAR SCIENCE AND ENGINEERING 165, 117 (2010)
          The 235U(n,f) Prompt Fission Neutron Spectrum at 100 K Input Neutron Energy
          CEA, France: D. Regnier, O. Litaize and O. Serot
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 59-65
          Monte Carlo Simulation of Prompt Fission Gamma Emission
          IRMM; A. Al-Adili, F.-J. Hambsch, S. Pomp, and S. Oberstedt
          Peer-reviewed paper international journal
          Phys. Rev. C 86, 054601 – Published 5 November 2012
          Impact of prompt-neutron corrections on final fission-fragment distributions
          Romania, IRMM: A. Tudora, F.-J. Hambsch, S. Oberstedt
          Peer-reviewed paper international journal
          Nuclear Physics A, Volumes 890–891, 1 October 2012, Pages 77-101
          Sub-barrier resonance fission and its effects on fission fragment properties
          Germany, France: Karl-Heinz Schmidt, Beatriz Jurado
          Peer-reviewed paper international journal
          Phys. Rev. C 83, 014607 – Published 28 January 2011
          Thermodynamics of nuclei in thermal contact
          Germany, France: Karl-Heinz Schmidt, Beatriz Jurado
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 147-157
          Global view on fission observables – new insights and new puzzles
          Germany, France: Karl-Heinz Schmidt, Beatriz Jurado
          Peer-reviewed paper international journal
          Phys. Rev. C 83, 061601 – Published 29 June 2011
          Final excitation energy of fission fragments
          Germany, France: Karl-Heinz Schmidt, Beatriz Jurado
          Peer-reviewed paper international journal
          Phys. Rev. Lett. 104, 212501 – Published 25 May 2010
          Entropy Driven Excitation Energy Sorting in Superfluid Fission Dynamics
          CEA, France: D. Regnier, O. Litaize and O. Serot
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 59-65
          Monte Carlo Simulation of Prompt Fission Gamma Emission
          CEA, France; LANL, USA: Thierry Granier, Ronald O. Nelson, Thierry Ethvignot, Matthew Devlin, Nick Fotiades, Wallid Younes, Paul Garrett
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 185-190, ISSN 1875-3892
          Investigation of Prompt X-ray Emission in Fission
          IRMM: A. Al-Adili, F.-J. Hambsch, S. Pomp, S. Oberstedt
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 158-164
          Indication of anisotropic TKE and mass emission in 234U(n,f)
          Russia: A.S. Vorobyev, O.A. Shcherbakov, Yu.S. Pleva, A.M. Gagarski, G.V. Val'ski, G.A. Petrov, V.I. Petrova, T.A. Zavarukhina
          Peer-reviewed paper international journal
          Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Volume 598 (2009) 795-801.
          Measurements of angular and energy distributions of prompt neutrons from thermal neutron-induced fission
          CEA, France: O. Litaize and O. Serot
          Peer-reviewed paper international journal
          Phys. Rev. C 82, 054616 – Published 29 November 2010
          Investigation of phenomenological models for the Monte Carlo simulation of the prompt fission neutron and gamma emission
          LANL (USA): E. Kwan, C.Y. Wu, R.C. Haight, H.Y. Lee, T.A. Bredeweg, A. Chyzh, M. Devlin, N. Fotiades, J.M. Gostic, R.A. Henderson, M. Jandel, A. Laptev, R.O. Nelson, J.M. O'Donnell, B.A. Perdue, T.N. Taddeucci, J.L. Ullmann, S.A. Wender
          Peer-reviewed paper international journal
          Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Volume 688, 1 October 2012, Pages 55-61
          Prompt energy distribution of 235U(n,f) at bombarding energies of 1–20 MeV
          IRMM: Sh. Zeynalov, O.V. Zeynalova, F.-J. Hambsch, S. Oberstedt
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 132-140
          A new approach to prompt fission neutron TOF data treatment
          CEA (France) : Olivier Litaize, Olivier Serot, David Regnier, Stephane Theveny, Sebastien Onde,
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 51-58
          New Features of the FIFRELIN Code for the Investigation of Fission Fragments Characteristics
          IRMM: Sh. Zeynalov, O.V. Zeynalova, F.-J. Hambsch, S. Oberstedt
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 132-140
          A new approach to prompt fission neutron TOF data treatment
          Slovenia, Belorussia, Japan, IAEA: Ivan Kodeli, Andrej Trkov, Roberto Capote, Yasunobu Nagaya, Vladimir Maslov
          Peer-reviewed paper international journal
          Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Volume 610, Issue 2, 1 November 2009, Pages 540-552
          Evaluation and use of the prompt fission neutron spectrum and spectra covariance matrices in criticality and shielding
          Germany, France: Karl-Heinz Schmidt, Beatriz Jurado
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 147-157
          Global view on fission observables – new insights and new puzzles
          Germany, France: Karl-Heinz Schmidt, Beatriz Jurado
          Peer-reviewed paper international journal
          Phys. Rev. C 83, 014607 – Published 28 January 2011
          Thermodynamics of nuclei in thermal contact
          CEA, France; LANL, USA: Thierry Granier, Ronald O. Nelson, Thierry Ethvignot, Matthew Devlin, Nick Fotiades, Wallid Younes, Paul Garrett
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 185-190, ISSN 1875-3892
          Investigation of Prompt X-ray Emission in Fission
          Romania, IRMM: A. Tudora, C. Morariu, F.-J. Hambsch, S. Oberstedt, C. Manailescu,
          Peer-reviewed paper international journal
          Physics Procedia, Volume 31, 2012, Pages 43-50
          Prompt Gamma-ray Energy in the Frame of Prompt Neutron Emission Models
          LLNL, USA; R. Vogt, J. Randrup, D. A. Brown, M. A. Descalle, and W. E. Ormand
          Peer-reviewed paper international journal
          Phys. Rev. C 85, 024608 – Published 13 February 2012
          Event-by-event evaluation of the prompt fission neutron spectrum from 239Pu(n,f)
          LANL (USA): Patrick Talou, Mike Rising, Toshihiko Kawano and Anil Prinja
          Peer-reviewed paper international journal
          EPJ Web of Conferences 27, 00001 (2012)
          Systematic Quantification of Uncertainties for Evaluated Prompt Fission Neutron Spectra and Multiplicities
          LANL, USA and RPI, USA: P. Talou, B. Becker, T. Kawano, M. B. Chadwick, and Y. Danon
          Peer-reviewed paper international journal
          Phys. Rev. C 83, 064612 – Published 23 June 2011
          Advanced Monte Carlo modeling of prompt fission neutrons for thermal and fast neutron-induced fission reactions on 239Pu
          CEA, France: O. Litaize and O. Serot
          Peer-reviewed paper international journal
          Phys. Rev. C 82, 054616 – Published 29 November 2010
          Investigation of phenomenological models for the Monte Carlo simulation of the prompt fission neutron and gamma emission
          Romania, IRMM: C. Manailescu, A. Tudora, F.-J. Hambsch, C. Morariu, S. Oberstedt
          Peer-reviewed paper international journal
          Nuclear Physics A, Volume 867, Issue 1, 1 October 2011, Pages 12-40
          Possible reference method of total excitation energy partition between complementary fission fragments
          LANL (USA): P. Talou, P.G. Young, T. Kawano, M. Rising, M.B. Chadwick
          Peer-reviewed paper international journal
          Nuclear Data Sheets, Volume 112, Issue 12, December 2011, Pages 3054-3074,
          Quantification of Uncertainties for Evaluated Neutron-Induced Reactions on Actinides in the Fast Energy Range
          LANL, USA and RPI, USA: P. Talou, B. Becker, T. Kawano, M. B. Chadwick, and Y. Danon
          Peer-reviewed paper international journal
          Phys. Rev. C 83, 064612 – Published 23 June 2011
          Advanced Monte Carlo modeling of prompt fission neutrons for thermal and fast neutron-induced fission reactions on 239Pu
          LANL, USA and CEA, France: S. Noda, R. C. Haight, R. O. Nelson, M. Devlin, J. M. O’Donnell, A. Chatillon, T. Granier, G. Bélier, J. Taieb, T. Kawano, and P. Talou
          Peer-reviewed paper international journal
          Phys. Rev. C 83, 034604 – Published 10 March 2011
          Prompt fission neutron spectra from fission induced by 1 to 8 MeV neutrons on U-235 and Pu-239 using the double time-of-flight technique
          Russia: A.S. Vorobyev, O.A. Shcherbakov, Yu.S. Pleva, A.M. Gagarski, G.V. Val'ski, G.A. Petrov, V.I. Petrova, T.A. Zavarukhina
          Peer-reviewed paper international journal
          Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Volume 598 (2009) 795-801.
          Measurements of angular and energy distributions of prompt neutrons from thermal neutron-induced fission
          Germany, France: Karl-Heinz Schmidt, Beatriz Jurado
          Peer-reviewed paper international journal
          Phys. Rev. Lett. 104, 212501 – Published 25 May 2010
          Entropy Driven Excitation Energy Sorting in Superfluid Fission Dynamics
          Germany, France: Karl-Heinz Schmidt, Beatriz Jurado
          Peer-reviewed paper international journal
          Phys. Rev. C 83, 061601 – Published 29 June 2011
          Final excitation energy of fission fragments
          LLNL, USA; R. Vogt, J. Randrup, D. A. Brown, M. A. Descalle, and W. E. Ormand
          Peer-reviewed paper international journal
          Phys. Rev. C 85, 024608 – Published 13 February 2012
          Event-by-event evaluation of the prompt fission neutron spectrum from 239Pu(n,f)
          IRMM and Ohio University, USA:
          Peer-reviewed paper international journal
          NUCLEAR SCIENCE AND ENGINEERING: 168, 73–74 (2011)
          Absolute Ratio 252Cf to 235U Prompt Fission Neutron Spectra
          LANL, USA and CEA, France: S. Noda, R. C. Haight, R. O. Nelson, M. Devlin, J. M. O’Donnell, A. Chatillon, T. Granier, G. Bélier, J. Taieb, T. Kawano, and P. Talou
          Peer-reviewed paper international journal
          Phys. Rev. C 83, 034604 – Published 10 March 2011
          Prompt fission neutron spectra from fission induced by 1 to 8 MeV neutrons on U-235 and Pu-239 using the double time-of-flight technique
          LANL (USA): P. Talou, P.G. Young, T. Kawano, M. Rising, M.B. Chadwick
          Peer-reviewed paper international journal
          Nuclear Data Sheets, Volume 112, Issue 12, December 2011, Pages 3054-3074,
          Quantification of Uncertainties for Evaluated Neutron-Induced Reactions on Actinides in the Fast Energy Range
          Slovenia, Belorussia, Japan, IAEA: Ivan Kodeli, Andrej Trkov, Roberto Capote, Yasunobu Nagaya, Vladimir Maslov
          Peer-reviewed paper international journal
          Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Volume 610, Issue 2, 1 November 2009, Pages 540-552
          Evaluation and use of the prompt fission neutron spectrum and spectra covariance matrices in criticality and shielding

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